Combining Chemical and Dynamical Measurements to Delineate the Interplay
between Dynamical Forcings and Global Pollution
Abstract
This work addresses the relationship between major dynamical forcings
and variability in NO column measurements. The dominating impact on
Siberia is due to El Niño, on Indonesia, Northern Australia and South
America is due to IOD,and on the remaining regions is due to NAO. That
NO pollution in Indonesia is modulated by IOD contradicts previous work
using AOD and El Niño. Simultaneous impacts of present and lagged
forcings are derived using multi-linear regression, demonstrating El
Niño impacts NO variability from 7 to 98 weeks ahead, while IOD and NAO
are mostly impacted by past changes in NO variability. In all cases,
lagged forcings exhibit more impact than present forcings, hinting at
non-linearity. Finally, dynamical forcings are responsible for over 50%
of the NO variability in most non-urban areas and over 40% in urban
Indonesia and China. These results demonstrate the significance of
climate forcing on short-lived air pollutants.