Laure Resplandy

and 34 more

The coastal ocean contributes to regulating atmospheric greenhouse gas concentrations by taking up carbon dioxide (CO2) and releasing nitrous oxide (N2O) and methane (CH4). Major advances have improved our understanding of the coastal air-sea exchanges of these three gasses since the first phase of the Regional Carbon Cycle Assessment and Processes (RECCAP in 2013), but a comprehensive view that integrates the three gasses at the global scale is still lacking. In this second phase (RECCAP2), we quantify global coastal ocean fluxes of CO2, N2O and CH4 using an ensemble of global gap-filled observation-based products and ocean biogeochemical models. The global coastal ocean is a net sink of CO2 in both observational products and models, but the magnitude of the median net global coastal uptake is ~60% larger in models (-0.72 vs. -0.44 PgC/yr, 1998-2018, coastal ocean area of 77 million km2). We attribute most of this model-product difference to the seasonality in sea surface CO2 partial pressure at mid- and high-latitudes, where models simulate stronger winter CO2 uptake. The global coastal ocean is a major source of N2O (+0.70 PgCO2-e /yr in observational product and +0.54 PgCO2-e /yr in model median) and of CH4 (+0.21 PgCO2-e /yr in observational product), which offsets a substantial proportion of the net radiative effect of coastal \co uptake (35-58% in CO2-equivalents). Data products and models need improvement to better resolve the spatio-temporal variability and long term trends in CO2, N2O and CH4 in the global coastal ocean.

Holly Olivarez

and 8 more

We use a statistical emulation technique to construct synthetic ensembles of global and regional sea-air carbon dioxide (CO2) flux from four observation-based products over 1985-2014. Much like ensembles of Earth system models that are constructed by perturbing their initial conditions, our synthetic ensemble members exhibit different phasing of internal variability and a common externally forced signal. Our synthetic ensembles illustrate an important role for internal variability in the temporal evolution of global and regional CO2 flux and produce a wide range of possible trends over 1990-1999 and 2000-2009. We assume a specific externally forced signal and calculate the likelihood of the observed trend given the distribution of synthetic trends during these two periods. Over the decade 1990-1999, three of the four observation-based products exhibit small negative trends in globally integrated sea-air CO2 flux (i.e., enhanced ocean CO2 absorption with time) that are highly probable (44-72% chance of occurrence) in their respective synthetic trend distributions. Over the decade 2000-2009, however, three of the four products show large negative trends in globally integrated sea-air CO2 flux that are somewhat improbable (17-19% chance of occurrence). Our synthetic ensembles suggest that the largest observation-based positive trends in global and Southern Ocean CO2 flux over 1990-1999 and the largest negative trends over 2000-2009 are somewhat improbable (<30% chance of occurrence). Our approach provides a new understanding of the role of internal and external processes in driving sea-air CO2 flux variability.