Baptiste Testa

and 11 more

Here we present a multi-season study of ice nucleating particles (INPs) active via the immersion freezing mechanism, which took place in north central Argentina, a worldwide hotspot for mesoscale convective storms. INPs were measured untreated, after heating to 95 °C, and after hydrogen peroxide digestion. No seasonal cycle of INP concentrations was observed. Biological INPs (denatured by heat) dominated the population active at -5 to -20 °C, while non-heat-labile organic INPs (decomposed by peroxide) dominated at lower temperatures, from -20 to -28 °C. Inorganic INPs (remaining after peroxide digestion), were minor contributors to the overall INP activity. Biological INP concentration active around -12 °C peaked during rain events and under high relative humidity, reflecting emission mechanisms independent of the background aerosol concentration. The ratio of non-heat-labile organic and inorganic INPs was generally constant, suggesting they originated from the same source, presumably from regional arable topsoil based on air mass histories. Single particle mass spectrometry showed that soil particles aerosolized from a regionally-common agricultural topsoil contained known mineral INP sources (K-feldspar and illite) as well as a significant organic component. The INP activity observed in this study correlates well with agricultural soil INP activities from this and other regions of the world, suggesting that the observed INP spectra might be typical of many arable landscapes. These results demonstrate the strong influence of regional continental landscapes, emitting INPs of types that are not yet well represented in global models.

Bjorn Stevens

and 291 more

The science guiding the \EURECA campaign and its measurements are presented. \EURECA comprised roughly five weeks of measurements in the downstream winter trades of the North Atlantic — eastward and south-eastward of Barbados. Through its ability to characterize processes operating across a wide range of scales, \EURECA marked a turning point in our ability to observationally study factors influencing clouds in the trades, how they will respond to warming, and their link to other components of the earth system, such as upper-ocean processes or, or the life-cycle of particulate matter. This characterization was made possible by thousands (2500) of sondes distributed to measure circulations on meso (200 km) and larger (500 km) scales, roughly four hundred hours of flight time by four heavily instrumented research aircraft, four global-ocean class research vessels, an advanced ground-based cloud observatory, a flotilla of autonomous or tethered measurement devices operating in the upper ocean (nearly 10000 profiles), lower atmosphere (continuous profiling), and along the air-sea interface, a network of water stable isotopologue measurements, complemented by special programmes of satellite remote sensing and modeling with a new generation of weather/climate models. In addition to providing an outline of the novel measurements and their composition into a unified and coordinated campaign, the six distinct scientific facets that \EURECA explored — from Brazil Ring Current Eddies to turbulence induced clustering of cloud droplets and its influence on warm-rain formation — are presented along with an overview \EURECA’s outreach activities, environmental impact, and guidelines for scientific practice.