Dust emissions related to anthropogenic activities (i.e., anthropogenic dust (AD)) is not represented in most global climate models and its radiative impact remains unassessed. In this study, we develop a new and physically based method to parameterize AD emission based on the DOE’s Energy Exascale Earth System Model version 1 (E3SMv1). This method relates AD emission to the crop land use fraction in the E3SMv1 land component. Major AD sources simulated by our parameterization include those over Central America, the Sahel, North India, and North China. The annual averaged AD emission is 567 Tg yr-1 in present-day (year 2000), which contributes to 13.3 % of total dust emission. Model evaluation against satellite and ground-based observations shows that the new parameterization can represent AD emissions and global dust cycle reasonably well. We find that the total dust emission increases by 13 % (495 Tg yr-1) from 1850 to 2000 mainly due to the cropland land use fraction changes, which induces a net dust direct effective radiative forcing of -0.041 W m-2 at top of the atmosphere. This AD-induced cooling exceeds 10% of the total anthropogenic aerosol direct effective radiative forcing from 1750 to 2014 estimated by the Intergovernmental Panel on Climate Change Sixth Assessment Report. Our findings indicate an important role of AD in the regional and global climate changes, which should be included in future climate change assessments.

Nitrate aerosol plays an important role in affecting regional air quality as well as Earth’s climate. However, it is not well represented or even neglected in many global climate models. In this study, we couple the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC) module with the four-mode version of the Modal Aerosol Module (MAM4) in DOE’s Energy Exascale Earth System Model version 2 (E3SMv2) to treat nitrate aerosol and its radiative effects. We find that nitrate aerosol simulated by E3SMv2-MAM4-MOSAIC is sensitive to the treatment of gaseous HNO3 transfer to/from interstitial particles related to accommodation coefficients of HNO3 (αHNO3) on dust and non-dust particles. We compare three different treatments of HNO3 transfer: 1) a treatment (MTC_SLOW) that uses a low αHNO3 in the mass transfer coefficient (MTC) calculation; 2) a dust-weighted MTC treatment (MTC_WGT) that uses a high αHNO3 on non-dust particles; and 3) a dust-weighted MTC treatment that also splits coarse mode aerosols into the coarse dust and sea salt sub-modes in MOSAIC (MTC_SPLC). MTC_WGT and MTC_SPLC increase the global annual mean (2005-2014) nitrate burden from 0.096 (MTC_SLOW) to 0.237 and 0.185 Tg N, respectively, mostly in the coarse mode. They also produce stronger nitrate direct radiative forcing (–0.048 and –0.051 W m–2, respectively) and indirect forcing (–0.33 and –0.35 W m–2, respectively) than MTC_SLOW (–0.021 and –0.24 W m–2). All three treatments overestimate nitrate surface concentrations compared with ground-based observations. MTC_WGT and MTC_SPLC improve the vertical profiles of nitrate concentrations against aircraft measurements below 400 hPa.