Harmonizing aerosol model parameters with retrieval property
assumptions: BrC as a case study
Abstract
Brown carbon (BrC) is an absorbing organic aerosol, primarily emitted
through biomass burning (BB), with a large degree of variability in
observed chemical and microphysical properties. This makes model
representation of the species difficult. Retrievals of BrC from measured
radiance fields have the potential to constrain model schemes and
improve estimates of BrC radiative effects. We used a retrieval of BrC
optical depth and mass from AERONET sites in BB regions to evaluate GISS
ModelE Earth system model’s BrC module. We approached this evaluation by
comparing BrC properties defined in ModelE with underlying properties
prescribed by the AERONET retrieval, then constrained our scheme to
match those assumptions. Our analysis showed that, just with this
initial harmonization, model bias was decreased, and performance,
relative to the retrieval, was improved. This allowed for an estimate of
global average BrC radiative effect, 0.03 Wm-2, grounded in the measured
radiance fields represented by the retrieval. Through this work, we
demonstrate the necessity of harmonizing model scheme parameters with a
speciated retrieval’s assumptions, even if such assumptions are not
necessarily more physically correct, to ensure an “apples-to-apples”
comparison and ultimately improve the estimate of individual aerosol
direct effects within a climate model.