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A highly integrated ceramic membrane-based reactor for intensifying the biomass gasification to clean syngas
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  • Wei Wei,
  • Qiaoqiao Zhou,
  • Ajing Ding,
  • Shuncheng Li,
  • Feng Zeng,
  • Xuerui Wang,
  • Chong Tian,
  • Zhaoxiang Zhong,
  • Huanhao Chen,
  • Xuehong Gu
Wei Wei
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Qiaoqiao Zhou
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Ajing Ding
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Shuncheng Li
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Feng Zeng
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Xuerui Wang
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Chong Tian
Liaoning Academy of Materials
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Zhaoxiang Zhong
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Huanhao Chen
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering
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Xuehong Gu
Nanjing Tech University State Key Laboratory of Materials-Oriented Chemical Engineering

Corresponding Author:[email protected]

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Abstract

Biomass gasification for syngas production is one of key operating units in the biomass utilization process, however its overall efficiency and stability are normally limited by the presence of complex impurities including particulate matters (PMs) and tars. Herein, a highly integrated ceramic membrane-based reactor was developed for high temperature syngas cleaning to allow the efficient in situ removal of PMs and tars from bio-vapours generated by biomass gasification. In specific, silicon carbide (SiC) membrane could in situ separate the PMs from biomass volatiles, while structured Ni 15La 5/S1-SiC catalyst (nickel and lanthanum-laden silicalite-1 zeolite supported on SiC foam) could promote the catalytic reforming of tars. Compared to other control reactors (i.e., with either membrane or catalyst alone), the integrated reactor demonstrated synergistic intensification in producing clean syngas from biomass gasification, with PM and tar removal efficiencies up to ~97% and ~90%, respectively, and excellent stability in five-cycle evaluations at 800 °C.
Submitted to AIChE Journal
27 May 2024Review(s) Completed, Editorial Evaluation Pending
27 May 2024Submission Checks Completed
27 May 2024Assigned to Editor
31 May 2024Reviewer(s) Assigned
23 Jun 2024Editorial Decision: Revise Major
23 Jul 20241st Revision Received
27 Jul 2024Submission Checks Completed
27 Jul 2024Assigned to Editor
27 Jul 2024Review(s) Completed, Editorial Evaluation Pending
27 Jul 2024Reviewer(s) Assigned
27 Aug 2024Editorial Decision: Revise Minor