Low marine clouds are a major source of uncertainty in cloud feedbacks across climate models and in forcing by aerosol-cloud interactions. The evolution of these clouds and their response to aerosol are sensitive to the ambient environmental conditions, so it is important to be able to determine different responses over a representative set of conditions. Here, we propose a novel approach to encompassing the broad range of conditions present in low marine cloud regions, by building a library of observed environmental conditions. This approach can be used, for example, to more systematically test the fidelity of Large Eddy Simulations (LES) in representing these clouds. ERA5 reanalysis and various satellite observations are used to extract and derive macrophysical and microphysical cloud-controlling variables (CCVs) such as SST, estimated inversion strength (EIS), subsidence, and cloud droplet number concentrations. A few locations in the stratocumulus (Sc) deck region of the Northeast Pacific during summer are selected to fill out a phase space of CCVs. Thereafter, Principal Component Analysis (PCA) is applied to reduce the dimensionality and to select a reduced set of components that explain most of the variability among CCVs in order to efficiently select cases for LES simulations that encompass the observed CCV phase space. From this phase space, 75-100 cases with distinct environmental conditions will be selected and used to initialize 2-day LES modeling to provide a spectrum of aerosol-cloud interactions and Sc-to-Cumulus transition under observed ambient conditions. Such a large number of simulations will help create statistics to assess how well the LES can simulate the cloud lifecycle when constrained by the ‘best estimate’ of the environmental conditions, and how sensitive the modeled clouds are to changes in these driving fields.

Observed stratocumulus to cumulus transitions (SCT) and their sensitivity to aerosols are studied using a Large-Eddy Simulation (LES) model that simulates the aerosol lifecycle, including aerosol sources and sinks. To initialize, force, and evaluate the LES, we used a combination of reanalysis, satellite, and aircraft data from the 2015 Cloud System Evolution in the Trades field campaign over the Northeast Pacific. The simulations follow two Lagrangian trajectories from initially overcast stratocumulus to the tropical shallow cumulus region near Hawaii. The first trajectory is characterized by an initially clean, well-mixed stratocumulus-topped marine boundary layer (MBL), then continuous MBL deepening and precipitation onset followed by a clear SCT and a consistent reduction of aerosols that ultimately leads to an ultra-clean layer in the upper MBL. The second trajectory is characterized by an initially polluted and decoupled MBL, weak precipitation, and a late SCT. Overall, the LES simulates the observed general MBL features. Sensitivity studies with different aerosol initial and boundary conditions reveal aerosol-induced changes in the transition, and albedo changes are decomposed into the Twomey effect and adjustments of cloud liquid water path and cloud fraction. Impacts on precipitation play a key role in the sensitivity to aerosols: for the first case, runs with enhanced aerosols exhibit distinct changes in microphysics and macrophysics such as enhanced cloud droplet number concentration, reduced precipitation, and delayed SCT. Cloud adjustments are dominant in this case. For the second case, enhancing aerosols does not affect cloud macrophysical properties significantly, and the Twomey effect dominates.