Greenhouse gasses (GHGs) play an important role in controlling local air pollution as well as climate change. In the present study, we retrieved column-averaged dry-air (X) mole fractions of carbon dioxide (CO2), methane (CH4), and carbon monoxide (CO) using a ground-based EM27/SUN Fourier Transform Infrared Spectrometer (FTIR). The EM27/SUN spectrometers are widely in use in the COllaborative Carbon Column Observing Network (COCCON). The PROFFAST software provided by COCCON has been used to analyze the measured atmospheric solar absorption spectra. In this paper, the diurnal variation and the time series of daily averaged XCO2, XCH4, and XCO covering the period December 2020 to May 2021 are analyzed. The maximum values of XCO2, XCH4, and XCO are observed to be 420.57 ppm, 1.93 ppm, and 170.40 ppb respectively. Less diurnal (XCO2 ~0.44 ppm; XCH4=0.004 ppm, and XCO=4.84 ppb) but clear seasonal changes are observed during the study period. The XCH4 and XCO from the Sentinel-5Precursor (S5P)/TROPOspheric Monitoring Instrument (TROPOMI) are compared against the EM27/SUN retrievals. The correlation coefficient ‘r’ between the EM27/SUN retrieved XCH4 and XCO against S5P/TROPOMI are 0.75 and 0.94 respectively.

Top-down estimates of CO2 fluxes are typically constrained by either surface-based or space-based CO2 observations. Both of these measurement types have spatial and temporal gaps in observational coverage that can lead to biases in inferred fluxes. Assimilating both surface-based and space-based measurements concurrently in a flux inversion framework improves observational coverage and reduces sampling biases. This study examines the consistency of flux constraints provided by these different observations and the potential to combine them by performing a series of six-year (2010–2015) CO2 flux inversions. Flux inversions are performed assimilating surface-based measurements from the in situ and flask network, measurements from the Total Carbon Column Observing Network (TCCON), and space-based measurements from the Greenhouse Gases Observing Satellite (GOSAT), or all three datasets combined. Combining the datasets results in more precise flux estimates for sub-continental regions relative to any of the datasets alone. Combining the datasets also improves the accuracy of the posterior fluxes, based on reduced root-mean-square differences between posterior-flux-simulated CO2 and aircraft-based CO2 over midlatitude regions (0.35–0.50~ppm) in comparison to GOSAT (0.39–0.57~ppm), TCCON (0.52–0.63~ppm), or in situ and flask measurements (0.45–0.53~ppm) alone. These results suggest that surface-based and GOSAT measurements give complementary constraints on CO2 fluxes in the northern extratropics and can be combined in flux inversions to improve observational coverage. This stands in contrast with many earlier attempts to combine these datasets and suggests that improvements in the NASA Atmospheric CO2 Observations from Space (ACOS) retrieval algorithm have significantly improved the consistency of space-based and surface-based flux constraints.