Satellite retrieval of cloud condensation nuclei concentrations in
marine stratocumulus by using clouds as CCN chambers
Abstract
A new methodology for satellite retrieval of cloud condensation nuclei
(CCN) in shallow marine boundary layer clouds is developed and validated
in this study. The methodology is based on retrieving cloud base drop
concentrations (Nd) and updrafts (Wb), and calculating the
supersaturation (S) based on that. Then Nd is the CCN at S. 50 The
accuracy of the satellite retrievals was validated against ship borne
measurements of CCN done in recent campaigns in the Southern Oceans
(ACE-SPACE, MARCUS & PEGASO [2015-2018]) and in the subtropics
(MAGIC [2012-2013]). The satellite retrieve Nd and S at cloud base
was related to the actually measured CCN(S) at sea surface. The main
findings show that: (a) coupled clouds have good agreement 55 between
satellite retrievals and ship measurements of CCN(S); (b) the best
agreement is achieved when using the brightest 10% of the clouds, and
accounting for their adiabatic fraction, as measured by aircrafts; (c)
most of the decoupled clouds had much lower CCN(S) than at the
underlying surface. This means that most CCN originate from the surface
and not from the free troposphere. This validates the satellite
retrievals and 60 allows us to further quantify the relationships
between CCN(S) and cloud microphysical properties.