Quantifying the contributions of atmospheric processes and meteorology
to severe PM2.5 pollution episodes during the COVID-19 lockdown in the
Beijing-Tianjin-Hebei, China
Abstract
A major tool for curtailing the spread of COVID-19 pandemic in China was
a nationwide lockdown, which led to significant reductions in
anthropogenic emissions and fine particulate matter (PM2.5). However,
the lockdown measures did not prevent high PM2.5 pollution episodes
(EPs). Three severe EPs were identified in the Beijing-Tianjin-Hebei
(BTH) region during the lockdown. The integrated process rate (IPR)
analysis tool in the Community Multiscale Air Quality (CMAQ) model was
employed to quantify the contributions of individual atmospheric
processes to PM2.5 formation during the lockdown in the BTH region. The
IPR results showed that emissions and aerosol processes were the
dominant sources of net surface PM2.5 in Beijing and Tianjin,
constituting a total of 86.2% and 92.9%, respectively, while
emissions, horizontal transport, and aerosol processes dominated the net
surface PM2.5 in Shijiazhuang and Baoding. In addition, the EPs in
Beijing and Tianjin were primarily driven by local emissions, while the
EPs in Shijiazhuang and Baoding were attributed to combined local
emissions and regional transport. The reductions in PM2.5 in Case 2
relative to Case 1 were attributed to the weaker PM2.5 formation from
emissions and aerosol processes. However, the EPs were enhanced by low
planetary boundary layer heights, low vertical export of PM2.5 from the
boundary layer to the free troposphere, and substantial horizontal
import, especially in Shijiazhuang and Baoding. This study improves the
understanding of buildup of PM2.5 during the EPs, and the results
provide insights for designing more effective emissions control
strategies to mitigate future PM2.5 episodes.