Atmospheric dust is a more extreme modifier of weather and climate on Mars than water vapor is on Earth. Global dust storms enshroud Mars in a veil of dust for months and have major implications for past and present climate, geologic history, habitability, and exploration. Yet their mysterious origins mean we remain unable to realistically simulate or predict them. In this White Paper, we find that key Knowledge Gaps are: A. how dust is lifted; B. constraints on near-surface winds and boundary-layer processes; C. the distribution of mobile surface dust; and D. the key processes and feedbacks by which dust storms begin and evolve. To make progress in the next decade, we make four Recommendations in order of priority: #1. Properly accommodate a minimum payload of meteorological and aeolian sensors on future Mars surface missions; #2. Continue orbital monitoring of the evolving surface dust distribution; #3. Expand orbital measurements to include winds and full diurnal coverage; and #4. Continue orbital monitoring and add surface measurements of aerosols during dust storms.